An entrance aperture of a GFCR system receives light from a scene of interest. The light is focused to form an image at a focal plane. Light associated with a selected field-of-view of the image at the focal plane is then confined to a spectral band at which a gas of interest absorbs. The confined light is split into first and second paths. A calibrating light is selectively produced from within the optical train at the focal plane. A portion of the calibrating light traverses each of the first and second paths. A region that is substantially non-interfering with respect to the spectral band is disposed in the first path. A gas cell filled with the gas of interest is disposed in the second path. The light passed through the region and through the gas cell is independently detected and used to generate output signals indicative of the light so-detected. The output signals are processed with the output signals generated by the light from the selected field-of-view of the image being used to generate a measure of the gas of interest and the output signals generated by the portion of the calibrating light traversing the first and second paths being used to calibrate the GFCR system.

An atmospheric refraction profile is determined using an imaging system positioned at a location that is simultaneously within line-of-sight of two celestial light sources. A variety of active or passive methods can be employed to cause the line-of-sight to vertically traverse through a refractive portion of an atmosphere. Images of the two celestial light sources are captured as the line-of-sight vertically traverses through the refractive portion of the atmosphere. Each such image indicates an apparent distance between the two celestial light sources. The apparent distances are used to determine refraction angles.